The set is a triple album of every Rolling Stones single—and their B-Sides—mostly in their original mono mixes (at least as of the 2002 reissue), in both the UK and US encompassing their entire era with Decca Records in the United Kingdom and London Records in the United States—hence the album's title.
The original collection was produced by Andrew Loog Oldham, and digitally compiled and prepared under his supervision by P. D. Rain and Jody Klein.
With a range from 1963 to 1971, the set begins with their very first UK single, Chuck Berry's "Come On", and runs to Sticky Fingers' "Brown Sugar" and "Wild Horses" (which Allen Klein shares release rights with The Rolling Stones).
CD1
01. Come On (1:48)
02. I Want To Be Loved (1:52)
03. I Wanna Be Your Man (1:43)
04. Stoned (2:09)
05. Not Fade Away (1:47)
06. Little By Little (2:39)
07. Its All Over Now (3:28)
08. Good Times, Bad Times (2:31)
09. Tell Me (3:48)
10. I Just Want To Make Love To You (2:17)
11. Time Is On My Side (2:53)
12. Congratulations (2:28)
13. Little Red Rooster (3:05)
14. Off The Hook (2:34)
15. Heart Of Stone (2:45)
16. What A Shame (3:02)
17. The Last Time (3:41)
18. Play With Fire (2:15)
19. (I Cant Get No) Satisfaction (3:44)
20. The Under Assistant West Coast Promotion Man (3:08)
21. The Spider And The Fly (3:38)
22. Get Off Of My Cloud (2:54)
23. Im Free (2:24)
24. The Singer Not The Song (2:24)
25. As Tears Go By (2:46)
CD2
01. Gotta Get Away (2:07)
02. 19th Nervous Breakdown (3:57)
03. Sad Day (3:03)
04. Paint It, Black (3:44)
05. Stupid Girl (2:56)
06. Long Long While (3:01)
07. Mothers Little Helper (2:45)
08. Lady Jane (3:11)
09. Have You Seen Your Mother, Baby, Standing In The Shadow? (2:34)
10. Whos Driving Your Plane? (3:14)
11. Lets Spend The Night Together (3:28)
12. Ruby Tuesday (3:13)
13. We Love You (4:37)
14. Dandelion (3:48)
15. Shes A Rainbow (4:12)
16. 2000 Light Years From Home (4:44)
17. In Another Land (2:53)
18. The Lantern (4:26)
19. Jumpin Jack Flash (3:37)
20. Child Of The Moon (rmk) (3:13)
CD3
01. Street Fighting Man (3:09)
02. No Expectations (3:55)
03. Surprise, Surprise (2:30)
04. Honky Tonk Women (3:01)
05. You Cant Always Get What You Want (4:49)
06. Memo From Turner (4:07)
07. Brown Sugar (3:49)
08. Wild Horses (5:41)
09. I Dont Know Why (Aka Dont Know Why I Love You) (3:02)
10. Try A Little Harder (2:17)
11. Out Of Time (3:22)
12. Jiving Sister Fanny (3:20)
13. Sympathy For The Devil (6:17)
