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The discs are thematically broken into three categories: "Top 90 Time," "Solo Piano, Tribute Records, Country-Bluegrass, Movie Scores," and "By Request (Favorites and Best Songs)" (two CDs). A full third of the music is previously unreleased; many familiar tracks are presented as unreleased live versions rather than the original studio recordings, and the majority of the remaining tracks are from single b-sides, collaborations and/or tribute albums and movie soundtracks.
Some noteworthy collaborations include a piano-and-saxophone duet with Ornette Coleman and a performance with Roger Waters of Pink Floyd's "Comfortably Numb." The set also offers a number of excellent examples of Hornsby's re-inventiveness with his own compositions, particularly in a live setting, for instance three different versions of “The Valley Road” are included—a live "bluesy funk" version with the Noise Makers, a Grammy-winning bluegrass version with the Nitty Gritty Dirt Band, and "a loose and sloppy but totally grooving boogie" take with the Grateful Dead.
"Song H" was a new composition that was nominated for Best Pop Instrumental at the 2007 Grammy Awards.
All songs written by Bruce Hornsby, except where noted.
(*) denotes previously unreleased live version
(**) denotes previously unreleased track
Disc one: "Top 90 Time"'
- "The Way It Is" *
- "Mandolin Rain" (w/ J. Hornsby) *
- "The Valley Road" (w/ J. Hornsby) *
- "Jacob's Ladder" (w/ J. Hornsby) *
- "Nobody There But Me" (w/ Haden / J. Hornsby) *
- "The End of Innocence" (w/ Henley) *
- "Look out Any Window" (w/ J. Hornsby) *
- "Across the River" (w/ J. Hornsby) *
- "Lost Soul" *
- "Fields of Gray" > "That's Where It's At" (Campbell, Hooks, Tiven, Tiven) *
- "Walk in the Sun"
- "Gonna Be Some Changes Made" *
- "Dreamland"
Disc two: "Solo Piano, Tribute Records, Country-Bluegrass, Movie Songs"
- "Song A"
- "Song B"
- "Song C"
- "Song D"
- "Variations on Swan Song & Song D"
- "Song F"
- "Song H" **
- "Barcelona Mona"
- "Backhand" (Jarrett)
- "Jack Straw" (Hunter, Weir)
- "Madman Across the Water" (Elton John, Bernie Taupin)
- "Darlin' Cory" (traditional)
- "The Valley Road" (w/ J. Hornsby) – bluegrass version
- "Crown of Jewels" *
- "Big Stick"
- "The Valley Road" (w/ J. Hornsby) – performed live with the Grateful Dead *
- "Hop / Skip and Jump" (Coleman) **
- "Love Me Still" (w/ Stevens) *
- "Shadowland"
Disc three: "By Request" (Favorites and Best Songs)
- "The Show Goes On" *
- "Barren Ground" (w/ J. Hornsby)
- "A Night on the Town" (w/ J. Hornsby) *
- "Talk of the Town" *
- "Rainbow's Cadillac"
- "Pastures of Plenty"
- "Spider Fingers" > "Tempus Fugit" (Powell) *
- "White Wheeled Limousine" > "Long Black Veil" (Dill / Wilkin) *
- "King of the Hill" > "Twelve Tone Tune" (Evans) > "Mystery Train" (Parker / Phillips) *
Disc four: "By Request" Part 2
- "Resting Place"
- "Preacher in the Ring, Part I"
- "Preacher in the Ring, Part II"
- "Fortunate Son" > "Comfortably Numb" (Dave Gilmour, Roger Waters)" *
- "Sneaking Up on Boo Radley" *
- "Shadowhand" *
- "Sticks & Stones" *
- "The Chill"
- "The Good Life"
- "What the Hell Happened"
- "Hooray for Tom"
- "Candy Mountain Run" *